Cost-based comparison between membrane systems and chemical absorption processes for CO2 capture from flue gas.
- Autores
- Arias, Ana Marisa; Mores, Patricia Liliana; Scenna, Nicolás José; Caballero, José Antonio; Mussati, Miguel Ceferino; Mussati, Sergio Fabián
- Año de publicación
- 2019
- Idioma
- inglés
- Tipo de recurso
- artículo
- Estado
- versión publicada
- Descripción
- An optimization study of membrane-based separation systems for carbon dioxide capture from flue gas of power plants is conducted, considering the possibility of employing up to four stages and using diverse options to create the required driving force. By proposing a superstructure-based model, the number of stages, recycle options, use of feed compression and/or permeate vacuum, driving force distribution along each membrane stage, operating conditions and equipment sizes are simultaneously optimized in order to minimize the total annual cost at high capture ratios and purity targets. Thus, different optimal arrangements are obtained and the total cost is reduced in about 20% compared without employing vacuum. Besides the optimal number of stages diminishes with decreasing purity, but it is independent of the capture ratio. Also, the total cost decreases with the increase of the membrane permeance requiring lower values of operating pressure and membrane areas. Permeance values higher than 2400 GPU lead to lower number of stages and recycles for the same separation target. By contrast, a sensitivity analysis shows that the total cost increases with the increase of the electricity price, capacity factor, and capital recovery factor, which are the more influential parameters in the objective function. Despite new optimal operating and design conditions are obtained when these parameters vary, no modifications in the optimal arrangement are observed.
Universidad Tecnológica Nacional (UTN) Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET)
Fil: Arias, Ana Marisa . Consejo Nacional de investigaciones Científicas y Técnicas (CONICET). Instituto de Desarrollo y Diseño (INGAR) ; Argentina.
Fil: Mores, Patricia Liliana. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina.
Fil: Mores, Patricia Liliana. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina.
Fil: Scenna, Nicolás José. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina.
Fil: Scenna, Nicolás José. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina.
Fil: Caballero, José Antonio. University of Alicante. Department of Chemical Engineering ; España.
Fil: Mussati, Miguel Ceferino. Consejo Nacional de investigaciones Científicas y Técnicas (CONICET). Instituto de Desarrollo y Diseño (INGAR) ; Argentina.
Fil: Mussati, Sergio Fabián. Consejo Nacional de investigaciones Científicas y Técnicas (CONICET). Instituto de Desarrollo y Diseño (INGAR) ; Argentina.
Peer Reviewed - Materia
-
CO2 capture
Membrane superstructure
NLP
GAMS
vacuum pressure - Nivel de accesibilidad
- acceso abierto
- Condiciones de uso
- 2024-03-27T20:23:27Z
- Repositorio
.jpg)
- Institución
- Universidad Tecnológica Nacional
- OAI Identificador
- oai:ria.utn.edu.ar:20.500.12272/10225
Ver los metadatos del registro completo
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Cost-based comparison between membrane systems and chemical absorption processes for CO2 capture from flue gas.Arias, Ana MarisaMores, Patricia LilianaScenna, Nicolás JoséCaballero, José AntonioMussati, Miguel CeferinoMussati, Sergio FabiánCO2 captureMembrane superstructureNLPGAMSvacuum pressureAn optimization study of membrane-based separation systems for carbon dioxide capture from flue gas of power plants is conducted, considering the possibility of employing up to four stages and using diverse options to create the required driving force. By proposing a superstructure-based model, the number of stages, recycle options, use of feed compression and/or permeate vacuum, driving force distribution along each membrane stage, operating conditions and equipment sizes are simultaneously optimized in order to minimize the total annual cost at high capture ratios and purity targets. Thus, different optimal arrangements are obtained and the total cost is reduced in about 20% compared without employing vacuum. Besides the optimal number of stages diminishes with decreasing purity, but it is independent of the capture ratio. Also, the total cost decreases with the increase of the membrane permeance requiring lower values of operating pressure and membrane areas. Permeance values higher than 2400 GPU lead to lower number of stages and recycles for the same separation target. By contrast, a sensitivity analysis shows that the total cost increases with the increase of the electricity price, capacity factor, and capital recovery factor, which are the more influential parameters in the objective function. Despite new optimal operating and design conditions are obtained when these parameters vary, no modifications in the optimal arrangement are observed.Universidad Tecnológica Nacional (UTN) Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET)Fil: Arias, Ana Marisa . Consejo Nacional de investigaciones Científicas y Técnicas (CONICET). Instituto de Desarrollo y Diseño (INGAR) ; Argentina.Fil: Mores, Patricia Liliana. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina.Fil: Mores, Patricia Liliana. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina.Fil: Scenna, Nicolás José. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina.Fil: Scenna, Nicolás José. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina.Fil: Caballero, José Antonio. University of Alicante. Department of Chemical Engineering ; España.Fil: Mussati, Miguel Ceferino. Consejo Nacional de investigaciones Científicas y Técnicas (CONICET). Instituto de Desarrollo y Diseño (INGAR) ; Argentina.Fil: Mussati, Sergio Fabián. Consejo Nacional de investigaciones Científicas y Técnicas (CONICET). Instituto de Desarrollo y Diseño (INGAR) ; Argentina.Peer Reviewed2024-03-27T20:23:27Z2024-03-27T20:23:27Z2019-05-09info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articulopdfapplication/pdfInternational Journal of Greenhouse Gas Control, 86, 177-190.1750-5836http://hdl.handle.net/20.500.12272/10225https://doi.org/10.1016/j.ijggc.2019.04.021enginfo:eu-repo/semantics/openAccess2024-03-27T20:23:27Zhttp://creativecommons.org/licenses/by-nc-nd/4.0/Attribution-NonCommercial-NoDerivatives 4.0 InternacionalAcceso abierto, con fines de estudio e investigación. Siempre con la mención de los autores.reponame:Repositorio Institucional Abierto (UTN)instname:Universidad Tecnológica Nacional2026-09-24T12:45:57Zoai:ria.utn.edu.ar:20.500.12272/10225instacron:UTNInstitucionalhttp://ria.utn.edu.ar/Universidad públicaNo correspondehttp://ria.utn.edu.ar/oaigestionria@rec.utn.edu.ar; fsuarez@rec.utn.edu.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:a2026-09-24 12:45:58.424Repositorio Institucional Abierto (UTN) - Universidad Tecnológica Nacionalfalse |
| dc.title.none.fl_str_mv |
Cost-based comparison between membrane systems and chemical absorption processes for CO2 capture from flue gas. |
| title |
Cost-based comparison between membrane systems and chemical absorption processes for CO2 capture from flue gas. |
| spellingShingle |
Cost-based comparison between membrane systems and chemical absorption processes for CO2 capture from flue gas. Arias, Ana Marisa CO2 capture Membrane superstructure NLP GAMS vacuum pressure |
| title_short |
Cost-based comparison between membrane systems and chemical absorption processes for CO2 capture from flue gas. |
| title_full |
Cost-based comparison between membrane systems and chemical absorption processes for CO2 capture from flue gas. |
| title_fullStr |
Cost-based comparison between membrane systems and chemical absorption processes for CO2 capture from flue gas. |
| title_full_unstemmed |
Cost-based comparison between membrane systems and chemical absorption processes for CO2 capture from flue gas. |
| title_sort |
Cost-based comparison between membrane systems and chemical absorption processes for CO2 capture from flue gas. |
| dc.creator.none.fl_str_mv |
Arias, Ana Marisa Mores, Patricia Liliana Scenna, Nicolás José Caballero, José Antonio Mussati, Miguel Ceferino Mussati, Sergio Fabián |
| author |
Arias, Ana Marisa |
| author_facet |
Arias, Ana Marisa Mores, Patricia Liliana Scenna, Nicolás José Caballero, José Antonio Mussati, Miguel Ceferino Mussati, Sergio Fabián |
| author_role |
author |
| author2 |
Mores, Patricia Liliana Scenna, Nicolás José Caballero, José Antonio Mussati, Miguel Ceferino Mussati, Sergio Fabián |
| author2_role |
author author author author author |
| dc.subject.none.fl_str_mv |
CO2 capture Membrane superstructure NLP GAMS vacuum pressure |
| topic |
CO2 capture Membrane superstructure NLP GAMS vacuum pressure |
| dc.description.none.fl_txt_mv |
An optimization study of membrane-based separation systems for carbon dioxide capture from flue gas of power plants is conducted, considering the possibility of employing up to four stages and using diverse options to create the required driving force. By proposing a superstructure-based model, the number of stages, recycle options, use of feed compression and/or permeate vacuum, driving force distribution along each membrane stage, operating conditions and equipment sizes are simultaneously optimized in order to minimize the total annual cost at high capture ratios and purity targets. Thus, different optimal arrangements are obtained and the total cost is reduced in about 20% compared without employing vacuum. Besides the optimal number of stages diminishes with decreasing purity, but it is independent of the capture ratio. Also, the total cost decreases with the increase of the membrane permeance requiring lower values of operating pressure and membrane areas. Permeance values higher than 2400 GPU lead to lower number of stages and recycles for the same separation target. By contrast, a sensitivity analysis shows that the total cost increases with the increase of the electricity price, capacity factor, and capital recovery factor, which are the more influential parameters in the objective function. Despite new optimal operating and design conditions are obtained when these parameters vary, no modifications in the optimal arrangement are observed. Universidad Tecnológica Nacional (UTN) Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) Fil: Arias, Ana Marisa . Consejo Nacional de investigaciones Científicas y Técnicas (CONICET). Instituto de Desarrollo y Diseño (INGAR) ; Argentina. Fil: Mores, Patricia Liliana. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina. Fil: Mores, Patricia Liliana. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina. Fil: Scenna, Nicolás José. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina. Fil: Scenna, Nicolás José. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina. Fil: Caballero, José Antonio. University of Alicante. Department of Chemical Engineering ; España. Fil: Mussati, Miguel Ceferino. Consejo Nacional de investigaciones Científicas y Técnicas (CONICET). Instituto de Desarrollo y Diseño (INGAR) ; Argentina. Fil: Mussati, Sergio Fabián. Consejo Nacional de investigaciones Científicas y Técnicas (CONICET). Instituto de Desarrollo y Diseño (INGAR) ; Argentina. Peer Reviewed |
| description |
An optimization study of membrane-based separation systems for carbon dioxide capture from flue gas of power plants is conducted, considering the possibility of employing up to four stages and using diverse options to create the required driving force. By proposing a superstructure-based model, the number of stages, recycle options, use of feed compression and/or permeate vacuum, driving force distribution along each membrane stage, operating conditions and equipment sizes are simultaneously optimized in order to minimize the total annual cost at high capture ratios and purity targets. Thus, different optimal arrangements are obtained and the total cost is reduced in about 20% compared without employing vacuum. Besides the optimal number of stages diminishes with decreasing purity, but it is independent of the capture ratio. Also, the total cost decreases with the increase of the membrane permeance requiring lower values of operating pressure and membrane areas. Permeance values higher than 2400 GPU lead to lower number of stages and recycles for the same separation target. By contrast, a sensitivity analysis shows that the total cost increases with the increase of the electricity price, capacity factor, and capital recovery factor, which are the more influential parameters in the objective function. Despite new optimal operating and design conditions are obtained when these parameters vary, no modifications in the optimal arrangement are observed. |
| publishDate |
2019 |
| dc.date.none.fl_str_mv |
2019-05-09 2024-03-27T20:23:27Z 2024-03-27T20:23:27Z |
| dc.type.none.fl_str_mv |
info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion http://purl.org/coar/resource_type/c_6501 info:ar-repo/semantics/articulo |
| format |
article |
| status_str |
publishedVersion |
| dc.identifier.none.fl_str_mv |
International Journal of Greenhouse Gas Control, 86, 177-190. 1750-5836 http://hdl.handle.net/20.500.12272/10225 https://doi.org/10.1016/j.ijggc.2019.04.021 |
| identifier_str_mv |
International Journal of Greenhouse Gas Control, 86, 177-190. 1750-5836 |
| url |
http://hdl.handle.net/20.500.12272/10225 https://doi.org/10.1016/j.ijggc.2019.04.021 |
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eng |
| language |
eng |
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info:eu-repo/semantics/openAccess 2024-03-27T20:23:27Z http://creativecommons.org/licenses/by-nc-nd/4.0/ Attribution-NonCommercial-NoDerivatives 4.0 Internacional Acceso abierto, con fines de estudio e investigación. Siempre con la mención de los autores. |
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openAccess |
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2024-03-27T20:23:27Z http://creativecommons.org/licenses/by-nc-nd/4.0/ Attribution-NonCommercial-NoDerivatives 4.0 Internacional Acceso abierto, con fines de estudio e investigación. Siempre con la mención de los autores. |
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pdf application/pdf |
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