Water influence on total annual cost for CO2 separation through a two-stage membrane system.

Autores
Arias, Ana Marisa; Kraft, Romina Alejandra; Scenna, Nicolás José; Mores, Patricia Liliana
Año de publicación
2023
Idioma
inglés
Tipo de recurso
documento de conferencia
Estado
versión publicada
Descripción
Carbon capture remains as one of the most promising alternatives to mitigate flue gas impact from installed plants. Several alternatives are being studied with different development levels. Membranes have been employed for gas separation in diverse industries; its application for carbon capture has been largely discussed. The mayor drawback of this technology lies on the high-energy requirement for driving force generation and its liability when treating humid gas. As a first approach to CO2 separation, early works study binary gas mixtures as representative of flue gases. However, the presence of a little amount of H2O may affect the separation in ways that need to be explored. In this work, an analysis on the impact of H2O presence on the driving force and overall separation efficiency is carried out. A four- component flue gas mixture including H2O and 02 is considered for a more realistic approach. The process objective is to recover 90% of the incoming CO2 and deliver a high purity permeate. Here, a typical two-stage counter-current membrane system is studied (Figure 1). Each stage includes a feed compressor followed by a cooler, the first one is also connected to a vacuum pump on the permeate side and another cooler. An optimization program based on a previous model [1] modified to consider a four-component mixture is implemented in GAMS. Mass and energy transfer phenomena, investment and operative costs, among others, are represented by a set of algebraic equations. Three different driving force generation setups are considered: feed compression, permeate vacuum, or a combination of both. Total annual cost (TAC) is selected as objective function to assess all the trade-offs between investment and operative costs, contrasting and accounting H2O influence. The resulting optimal driving force generation strategy includes a combination of feed compression and permeate vacuum pumping, fulfilling a 90% CO2 recovery. In fact, the incidence of investment over TAC is much less pronounced than the costs related to energy consumption.
Universidad Tecnológica Nacional (UTN) Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET)
Fil: Arias, Ana Marisa. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina.
Fil: Arias, Ana Marisa. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina.
Fil: Kraft, Romina Alejandra. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina.
Fil: Kraft, Romina Alejandra. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina.
Fil: Scenna, Nicolás José. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina.
Fil: Scenna, Nicolás José. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina.
Fil: Mores, Patricia Liliana. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina.
Fil: Mores, Patricia Liliana. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina.
Materia
membrane separation
CO2 capture
water influence
optimization model
Nivel de accesibilidad
acceso abierto
Condiciones de uso
2024-03-18T18:29:24Z
Repositorio
Repositorio Institucional Abierto (UTN)
Institución
Universidad Tecnológica Nacional
OAI Identificador
oai:ria.utn.edu.ar:20.500.12272/9810
Acceder
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network_acronym_str RIAUTN
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spelling Water influence on total annual cost for CO2 separation through a two-stage membrane system.Arias, Ana MarisaKraft, Romina AlejandraScenna, Nicolás JoséMores, Patricia Lilianamembrane separationCO2 capturewater influenceoptimization modelCarbon capture remains as one of the most promising alternatives to mitigate flue gas impact from installed plants. Several alternatives are being studied with different development levels. Membranes have been employed for gas separation in diverse industries; its application for carbon capture has been largely discussed. The mayor drawback of this technology lies on the high-energy requirement for driving force generation and its liability when treating humid gas. As a first approach to CO2 separation, early works study binary gas mixtures as representative of flue gases. However, the presence of a little amount of H2O may affect the separation in ways that need to be explored. In this work, an analysis on the impact of H2O presence on the driving force and overall separation efficiency is carried out. A four- component flue gas mixture including H2O and 02 is considered for a more realistic approach. The process objective is to recover 90% of the incoming CO2 and deliver a high purity permeate. Here, a typical two-stage counter-current membrane system is studied (Figure 1). Each stage includes a feed compressor followed by a cooler, the first one is also connected to a vacuum pump on the permeate side and another cooler. An optimization program based on a previous model [1] modified to consider a four-component mixture is implemented in GAMS. Mass and energy transfer phenomena, investment and operative costs, among others, are represented by a set of algebraic equations. Three different driving force generation setups are considered: feed compression, permeate vacuum, or a combination of both. Total annual cost (TAC) is selected as objective function to assess all the trade-offs between investment and operative costs, contrasting and accounting H2O influence. The resulting optimal driving force generation strategy includes a combination of feed compression and permeate vacuum pumping, fulfilling a 90% CO2 recovery. In fact, the incidence of investment over TAC is much less pronounced than the costs related to energy consumption.Universidad Tecnológica Nacional (UTN) Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET)Fil: Arias, Ana Marisa. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina.Fil: Arias, Ana Marisa. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina.Fil: Kraft, Romina Alejandra. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina.Fil: Kraft, Romina Alejandra. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina.Fil: Scenna, Nicolás José. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina.Fil: Scenna, Nicolás José. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina.Fil: Mores, Patricia Liliana. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina.Fil: Mores, Patricia Liliana. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina.Asociación Argentina de Ingenieros Químicos/ Oscar Pagola2024-03-18T18:29:24Z2024-03-18T18:29:24Z2023-06info:eu-repo/semantics/conferenceObjectinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_5794info:ar-repo/semantics/documentoDeConferenciapdfapplication/pdfWCCE11 - 11th World Congress of Chemical Engineering2953-5565http://hdl.handle.net/20.500.12272/9810enginfo:eu-repo/semantics/openAccess2024-03-18T18:29:24Zhttp://creativecommons.org/licenses/by-nc-nd/4.0/Attribution-NonCommercial-NoDerivatives 4.0 InternacionalAcceso abierto, con fines de estudio e investigación .Siempre con la mención de los autores.reponame:Repositorio Institucional Abierto (UTN)instname:Universidad Tecnológica Nacional2026-09-24T12:45:11Zoai:ria.utn.edu.ar:20.500.12272/9810instacron:UTNInstitucionalhttp://ria.utn.edu.ar/Universidad públicaNo correspondehttp://ria.utn.edu.ar/oaigestionria@rec.utn.edu.ar; fsuarez@rec.utn.edu.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:a2026-09-24 12:45:12.851Repositorio Institucional Abierto (UTN) - Universidad Tecnológica Nacionalfalse
dc.title.none.fl_str_mv Water influence on total annual cost for CO2 separation through a two-stage membrane system.
title Water influence on total annual cost for CO2 separation through a two-stage membrane system.
spellingShingle Water influence on total annual cost for CO2 separation through a two-stage membrane system.
Arias, Ana Marisa
membrane separation
CO2 capture
water influence
optimization model
title_short Water influence on total annual cost for CO2 separation through a two-stage membrane system.
title_full Water influence on total annual cost for CO2 separation through a two-stage membrane system.
title_fullStr Water influence on total annual cost for CO2 separation through a two-stage membrane system.
title_full_unstemmed Water influence on total annual cost for CO2 separation through a two-stage membrane system.
title_sort Water influence on total annual cost for CO2 separation through a two-stage membrane system.
dc.creator.none.fl_str_mv Arias, Ana Marisa
Kraft, Romina Alejandra
Scenna, Nicolás José
Mores, Patricia Liliana
author Arias, Ana Marisa
author_facet Arias, Ana Marisa
Kraft, Romina Alejandra
Scenna, Nicolás José
Mores, Patricia Liliana
author_role author
author2 Kraft, Romina Alejandra
Scenna, Nicolás José
Mores, Patricia Liliana
author2_role author
author
author
dc.subject.none.fl_str_mv membrane separation
CO2 capture
water influence
optimization model
topic membrane separation
CO2 capture
water influence
optimization model
dc.description.none.fl_txt_mv Carbon capture remains as one of the most promising alternatives to mitigate flue gas impact from installed plants. Several alternatives are being studied with different development levels. Membranes have been employed for gas separation in diverse industries; its application for carbon capture has been largely discussed. The mayor drawback of this technology lies on the high-energy requirement for driving force generation and its liability when treating humid gas. As a first approach to CO2 separation, early works study binary gas mixtures as representative of flue gases. However, the presence of a little amount of H2O may affect the separation in ways that need to be explored. In this work, an analysis on the impact of H2O presence on the driving force and overall separation efficiency is carried out. A four- component flue gas mixture including H2O and 02 is considered for a more realistic approach. The process objective is to recover 90% of the incoming CO2 and deliver a high purity permeate. Here, a typical two-stage counter-current membrane system is studied (Figure 1). Each stage includes a feed compressor followed by a cooler, the first one is also connected to a vacuum pump on the permeate side and another cooler. An optimization program based on a previous model [1] modified to consider a four-component mixture is implemented in GAMS. Mass and energy transfer phenomena, investment and operative costs, among others, are represented by a set of algebraic equations. Three different driving force generation setups are considered: feed compression, permeate vacuum, or a combination of both. Total annual cost (TAC) is selected as objective function to assess all the trade-offs between investment and operative costs, contrasting and accounting H2O influence. The resulting optimal driving force generation strategy includes a combination of feed compression and permeate vacuum pumping, fulfilling a 90% CO2 recovery. In fact, the incidence of investment over TAC is much less pronounced than the costs related to energy consumption.
Universidad Tecnológica Nacional (UTN) Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET)
Fil: Arias, Ana Marisa. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina.
Fil: Arias, Ana Marisa. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina.
Fil: Kraft, Romina Alejandra. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina.
Fil: Kraft, Romina Alejandra. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina.
Fil: Scenna, Nicolás José. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina.
Fil: Scenna, Nicolás José. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina.
Fil: Mores, Patricia Liliana. Universidad Tecnológica Nacional. Facultad Regional Rosario. Centro de Aplicaciones Informáticas y Modelado en Ingeniería (CAIMI) ; Argentina.
Fil: Mores, Patricia Liliana. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) ; Argentina.
description Carbon capture remains as one of the most promising alternatives to mitigate flue gas impact from installed plants. Several alternatives are being studied with different development levels. Membranes have been employed for gas separation in diverse industries; its application for carbon capture has been largely discussed. The mayor drawback of this technology lies on the high-energy requirement for driving force generation and its liability when treating humid gas. As a first approach to CO2 separation, early works study binary gas mixtures as representative of flue gases. However, the presence of a little amount of H2O may affect the separation in ways that need to be explored. In this work, an analysis on the impact of H2O presence on the driving force and overall separation efficiency is carried out. A four- component flue gas mixture including H2O and 02 is considered for a more realistic approach. The process objective is to recover 90% of the incoming CO2 and deliver a high purity permeate. Here, a typical two-stage counter-current membrane system is studied (Figure 1). Each stage includes a feed compressor followed by a cooler, the first one is also connected to a vacuum pump on the permeate side and another cooler. An optimization program based on a previous model [1] modified to consider a four-component mixture is implemented in GAMS. Mass and energy transfer phenomena, investment and operative costs, among others, are represented by a set of algebraic equations. Three different driving force generation setups are considered: feed compression, permeate vacuum, or a combination of both. Total annual cost (TAC) is selected as objective function to assess all the trade-offs between investment and operative costs, contrasting and accounting H2O influence. The resulting optimal driving force generation strategy includes a combination of feed compression and permeate vacuum pumping, fulfilling a 90% CO2 recovery. In fact, the incidence of investment over TAC is much less pronounced than the costs related to energy consumption.
publishDate 2023
dc.date.none.fl_str_mv 2023-06
2024-03-18T18:29:24Z
2024-03-18T18:29:24Z
dc.type.none.fl_str_mv info:eu-repo/semantics/conferenceObject
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_5794
info:ar-repo/semantics/documentoDeConferencia
format conferenceObject
status_str publishedVersion
dc.identifier.none.fl_str_mv WCCE11 - 11th World Congress of Chemical Engineering
2953-5565
http://hdl.handle.net/20.500.12272/9810
identifier_str_mv WCCE11 - 11th World Congress of Chemical Engineering
2953-5565
url http://hdl.handle.net/20.500.12272/9810
dc.language.none.fl_str_mv eng
language eng
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
2024-03-18T18:29:24Z
http://creativecommons.org/licenses/by-nc-nd/4.0/
Attribution-NonCommercial-NoDerivatives 4.0 Internacional
Acceso abierto, con fines de estudio e investigación .Siempre con la mención de los autores.
eu_rights_str_mv openAccess
rights_invalid_str_mv 2024-03-18T18:29:24Z
http://creativecommons.org/licenses/by-nc-nd/4.0/
Attribution-NonCommercial-NoDerivatives 4.0 Internacional
Acceso abierto, con fines de estudio e investigación .Siempre con la mención de los autores.
dc.format.none.fl_str_mv pdf
application/pdf
dc.publisher.none.fl_str_mv Asociación Argentina de Ingenieros Químicos/ Oscar Pagola
publisher.none.fl_str_mv Asociación Argentina de Ingenieros Químicos/ Oscar Pagola
dc.source.none.fl_str_mv reponame:Repositorio Institucional Abierto (UTN)
instname:Universidad Tecnológica Nacional
reponame_str Repositorio Institucional Abierto (UTN)
collection Repositorio Institucional Abierto (UTN)
instname_str Universidad Tecnológica Nacional
repository.name.fl_str_mv Repositorio Institucional Abierto (UTN) - Universidad Tecnológica Nacional
repository.mail.fl_str_mv gestionria@rec.utn.edu.ar; fsuarez@rec.utn.edu.ar
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