Determination of nanoscale mechanical properties of polymers via plasmonic nanoantennas

Autores
Boggiano, Hilario D.; Berté, Rodrigo; Cortés, Emiliano; Maier, Stefan A.; Bragas, Andrea V.; Scarpettini, Alberto Franco
Año de publicación
2020
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
Nanotechnology and the consequent emergence of miniaturized devices are driving the need to improve our understanding of the mechanical properties of a myriad of materials. Here we focus on amorphous polymeric materials and introduce a new way to determine the nanoscale mechanical response of polymeric thin films in the GHz range, using ultrafast optical means. Coupling of the films to plasmonic nanoantennas excited at their vibrational eigenfrequencies allows the extraction of the values of the mechanical moduli as well as the estimation of the glass transition temperature via time-domain measurements, here demonstrated for PMMA films. This nanoscale method can be extended to the determination of mechanical and elastic properties of a wide range of spatially strongly confined materials.
PICT 2017-2534, PIP 112 201301 00619, UBACyT Proyecto 20020170100432BA, PID-UTI4836, Deutsche Forschungsgemeinschaft (Germany’s Excellence Strategy, EXC 2089/1−390776260), European Commission, ERC-802989 (Catalight), EPSRC Reactive Plasmonics Programme (EP/M013812/1), Lee Lucas Chair in Physics.
Fil: Boggiano, Hilario D. Universidad de Buenos Aires. Departamento de Física, FCEN, IFIBA CONICET; Argentina.
Fil: : Berté, Rodrigo. Chair in Hybrid Nanosystems, Nanoinstitute Munich, Faculty of Physics, Ludwig-Maximilians-Universität München; Germany.
Fil: Scarpettini, Alberto Franco. Universidad Tecnológica Nacional. Facultad Regional Delta. Grupo de Fotónica Aplicada; Argentina.
Fil: Scarpettini, Alberto Franco. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET); Argentina.
Fil: Cortés, Emiliano. Nanoinstitute Munich. Faculty of Physics. Ludwig-Maximilians-Universität; Germany.
Fil: Maier, Stefan A. Chair in Hybrid Nanosystems. Nanoinstitute Munich. Faculty of Physics. Ludwig-Maximilians-Universität München; Germany
Fil: Maier, Stefan A. Department of Physics, Imperial College London; United Kingdom.
Fil: Bragas, Andrea V. CONICET. Universidad de Buenos Aires. Instituto de Física de Buenos Aires (IFIBA); Argentina.
Peer Reviewed
Fuente
ACS Photonics 7, 1403-1409 (2020)
Materia
Nanomechanics
Ultrafast optics
Nanoantennas
Polymers
Plasmonics
Nivel de accesibilidad
acceso abierto
Condiciones de uso
2024-03-18T21:50:21Z
Repositorio
Repositorio Institucional Abierto (UTN)
Institución
Universidad Tecnológica Nacional
OAI Identificador
oai:ria.utn.edu.ar:20.500.12272/9835
Acceder
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network_acronym_str RIAUTN
repository_id_str a
network_name_str Repositorio Institucional Abierto (UTN)
spelling Determination of nanoscale mechanical properties of polymers via plasmonic nanoantennasBoggiano, Hilario D.Berté, RodrigoCortés, EmilianoMaier, Stefan A.Bragas, Andrea V.Scarpettini, Alberto FrancoNanomechanicsUltrafast opticsNanoantennasPolymersPlasmonicsNanotechnology and the consequent emergence of miniaturized devices are driving the need to improve our understanding of the mechanical properties of a myriad of materials. Here we focus on amorphous polymeric materials and introduce a new way to determine the nanoscale mechanical response of polymeric thin films in the GHz range, using ultrafast optical means. Coupling of the films to plasmonic nanoantennas excited at their vibrational eigenfrequencies allows the extraction of the values of the mechanical moduli as well as the estimation of the glass transition temperature via time-domain measurements, here demonstrated for PMMA films. This nanoscale method can be extended to the determination of mechanical and elastic properties of a wide range of spatially strongly confined materials.PICT 2017-2534, PIP 112 201301 00619, UBACyT Proyecto 20020170100432BA, PID-UTI4836, Deutsche Forschungsgemeinschaft (Germany’s Excellence Strategy, EXC 2089/1−390776260), European Commission, ERC-802989 (Catalight), EPSRC Reactive Plasmonics Programme (EP/M013812/1), Lee Lucas Chair in Physics.Fil: Boggiano, Hilario D. Universidad de Buenos Aires. Departamento de Física, FCEN, IFIBA CONICET; Argentina.Fil: : Berté, Rodrigo. Chair in Hybrid Nanosystems, Nanoinstitute Munich, Faculty of Physics, Ludwig-Maximilians-Universität München; Germany.Fil: Scarpettini, Alberto Franco. Universidad Tecnológica Nacional. Facultad Regional Delta. Grupo de Fotónica Aplicada; Argentina.Fil: Scarpettini, Alberto Franco. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET); Argentina.Fil: Cortés, Emiliano. Nanoinstitute Munich. Faculty of Physics. Ludwig-Maximilians-Universität; Germany.Fil: Maier, Stefan A. Chair in Hybrid Nanosystems. Nanoinstitute Munich. Faculty of Physics. Ludwig-Maximilians-Universität München; GermanyFil: Maier, Stefan A. Department of Physics, Imperial College London; United Kingdom.Fil: Bragas, Andrea V. CONICET. Universidad de Buenos Aires. Instituto de Física de Buenos Aires (IFIBA); Argentina.Peer Reviewed2024-03-18T21:50:21Z2024-03-18T21:50:21Z2020-06-02info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articulopdfapplication/pdfACS Photonics (ISSN: 2330-4022) 7, 1403-1409 (2020)2330-4022http://hdl.handle.net/20.500.12272/9835ACS Photonics 7, 1403-1409 (2020)reponame:Repositorio Institucional Abierto (UTN)instname:Universidad Tecnológica Nacionalenghttps://pubs.acs.org/doi/10.1021/acsphotonics.0c00 631info:eu-repo/semantics/openAccess2024-03-18T21:50:21Zhttp://creativecommons.org/licenses/by/4.0/Atribución 4.0 InternacionalAmerican Chemical SocietyAtribución (by)2026-09-24T12:48:37Zoai:ria.utn.edu.ar:20.500.12272/9835instacron:UTNInstitucionalhttp://ria.utn.edu.ar/Universidad públicaNo correspondehttp://ria.utn.edu.ar/oaigestionria@rec.utn.edu.ar; fsuarez@rec.utn.edu.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:a2026-09-24 12:48:38.326Repositorio Institucional Abierto (UTN) - Universidad Tecnológica Nacionalfalse
dc.title.none.fl_str_mv Determination of nanoscale mechanical properties of polymers via plasmonic nanoantennas
title Determination of nanoscale mechanical properties of polymers via plasmonic nanoantennas
spellingShingle Determination of nanoscale mechanical properties of polymers via plasmonic nanoantennas
Boggiano, Hilario D.
Nanomechanics
Ultrafast optics
Nanoantennas
Polymers
Plasmonics
title_short Determination of nanoscale mechanical properties of polymers via plasmonic nanoantennas
title_full Determination of nanoscale mechanical properties of polymers via plasmonic nanoantennas
title_fullStr Determination of nanoscale mechanical properties of polymers via plasmonic nanoantennas
title_full_unstemmed Determination of nanoscale mechanical properties of polymers via plasmonic nanoantennas
title_sort Determination of nanoscale mechanical properties of polymers via plasmonic nanoantennas
dc.creator.none.fl_str_mv Boggiano, Hilario D.
Berté, Rodrigo
Cortés, Emiliano
Maier, Stefan A.
Bragas, Andrea V.
Scarpettini, Alberto Franco
author Boggiano, Hilario D.
author_facet Boggiano, Hilario D.
Berté, Rodrigo
Cortés, Emiliano
Maier, Stefan A.
Bragas, Andrea V.
Scarpettini, Alberto Franco
author_role author
author2 Berté, Rodrigo
Cortés, Emiliano
Maier, Stefan A.
Bragas, Andrea V.
Scarpettini, Alberto Franco
author2_role author
author
author
author
author
dc.subject.none.fl_str_mv Nanomechanics
Ultrafast optics
Nanoantennas
Polymers
Plasmonics
topic Nanomechanics
Ultrafast optics
Nanoantennas
Polymers
Plasmonics
dc.description.none.fl_txt_mv Nanotechnology and the consequent emergence of miniaturized devices are driving the need to improve our understanding of the mechanical properties of a myriad of materials. Here we focus on amorphous polymeric materials and introduce a new way to determine the nanoscale mechanical response of polymeric thin films in the GHz range, using ultrafast optical means. Coupling of the films to plasmonic nanoantennas excited at their vibrational eigenfrequencies allows the extraction of the values of the mechanical moduli as well as the estimation of the glass transition temperature via time-domain measurements, here demonstrated for PMMA films. This nanoscale method can be extended to the determination of mechanical and elastic properties of a wide range of spatially strongly confined materials.
PICT 2017-2534, PIP 112 201301 00619, UBACyT Proyecto 20020170100432BA, PID-UTI4836, Deutsche Forschungsgemeinschaft (Germany’s Excellence Strategy, EXC 2089/1−390776260), European Commission, ERC-802989 (Catalight), EPSRC Reactive Plasmonics Programme (EP/M013812/1), Lee Lucas Chair in Physics.
Fil: Boggiano, Hilario D. Universidad de Buenos Aires. Departamento de Física, FCEN, IFIBA CONICET; Argentina.
Fil: : Berté, Rodrigo. Chair in Hybrid Nanosystems, Nanoinstitute Munich, Faculty of Physics, Ludwig-Maximilians-Universität München; Germany.
Fil: Scarpettini, Alberto Franco. Universidad Tecnológica Nacional. Facultad Regional Delta. Grupo de Fotónica Aplicada; Argentina.
Fil: Scarpettini, Alberto Franco. Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET); Argentina.
Fil: Cortés, Emiliano. Nanoinstitute Munich. Faculty of Physics. Ludwig-Maximilians-Universität; Germany.
Fil: Maier, Stefan A. Chair in Hybrid Nanosystems. Nanoinstitute Munich. Faculty of Physics. Ludwig-Maximilians-Universität München; Germany
Fil: Maier, Stefan A. Department of Physics, Imperial College London; United Kingdom.
Fil: Bragas, Andrea V. CONICET. Universidad de Buenos Aires. Instituto de Física de Buenos Aires (IFIBA); Argentina.
Peer Reviewed
description Nanotechnology and the consequent emergence of miniaturized devices are driving the need to improve our understanding of the mechanical properties of a myriad of materials. Here we focus on amorphous polymeric materials and introduce a new way to determine the nanoscale mechanical response of polymeric thin films in the GHz range, using ultrafast optical means. Coupling of the films to plasmonic nanoantennas excited at their vibrational eigenfrequencies allows the extraction of the values of the mechanical moduli as well as the estimation of the glass transition temperature via time-domain measurements, here demonstrated for PMMA films. This nanoscale method can be extended to the determination of mechanical and elastic properties of a wide range of spatially strongly confined materials.
publishDate 2020
dc.date.none.fl_str_mv 2020-06-02
2024-03-18T21:50:21Z
2024-03-18T21:50:21Z
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv ACS Photonics (ISSN: 2330-4022) 7, 1403-1409 (2020)
2330-4022
http://hdl.handle.net/20.500.12272/9835
identifier_str_mv ACS Photonics (ISSN: 2330-4022) 7, 1403-1409 (2020)
2330-4022
url http://hdl.handle.net/20.500.12272/9835
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv https://pubs.acs.org/doi/10.1021/acsphotonics.0c00 631
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
2024-03-18T21:50:21Z
http://creativecommons.org/licenses/by/4.0/
Atribución 4.0 Internacional
American Chemical Society
Atribución (by)
eu_rights_str_mv openAccess
rights_invalid_str_mv 2024-03-18T21:50:21Z
http://creativecommons.org/licenses/by/4.0/
Atribución 4.0 Internacional
American Chemical Society
Atribución (by)
dc.format.none.fl_str_mv pdf
application/pdf
dc.source.none.fl_str_mv ACS Photonics 7, 1403-1409 (2020)
reponame:Repositorio Institucional Abierto (UTN)
instname:Universidad Tecnológica Nacional
reponame_str Repositorio Institucional Abierto (UTN)
collection Repositorio Institucional Abierto (UTN)
instname_str Universidad Tecnológica Nacional
repository.name.fl_str_mv Repositorio Institucional Abierto (UTN) - Universidad Tecnológica Nacional
repository.mail.fl_str_mv gestionria@rec.utn.edu.ar; fsuarez@rec.utn.edu.ar
_version_ 1877230969622102016
score 13.24418

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