Determination of Nanoscale Mechanical Properties of Polymers via Plasmonic Nanoantennas

Autores
Boggiano, Hilario D; Berté, Rodrigo; Scarpettini, Alberto F; Cortés, Emiliano; Maier, Stefan A.; Bragas, Andrea V.
Año de publicación
2020
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
Nanotechnology and the consequent emergence of miniaturized devices are driving the need to improve our understanding of the mechanical properties of a myriad of materials. Here we focus on amorphous polymeric materials and introduce a new way to determine the nanoscale mechanical response of polymeric thin films in the GHz range, using ultrafast optical means. Coupling of the films to plasmonic nanoantennas excited at their vibrational eigenfrequencies allows the extraction of the values of the mechanical moduli as well as the estimation of the glass transition temperature via time-domain measurements, here demonstrated for PMMA films. This nanoscale method can be extended to the determination of mechanical and elastic properties of a wide range of spatially strongly confined materials.
Fil: Scarpettini, Alberto F. Universidad Tecnológica Nacional. Facultad Regional Delta. Grupo Nanofotonica; Argentina.
Peer Reviewed
Materia
UTN
FRD
nanomechanics
ultrafast optics
nanoantennas
polymers
plasmonics
Nivel de accesibilidad
acceso abierto
Condiciones de uso
2020-09-18T18:27:36Z
Repositorio
Repositorio Institucional Abierto (UTN)
Institución
Universidad Tecnológica Nacional
OAI Identificador
oai:ria.utn.edu.ar:20.500.12272/4551

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network_acronym_str RIAUTN
repository_id_str a
network_name_str Repositorio Institucional Abierto (UTN)
spelling Determination of Nanoscale Mechanical Properties of Polymers via Plasmonic NanoantennasBoggiano, Hilario DBerté, RodrigoScarpettini, Alberto FCortés, EmilianoMaier, Stefan A.Bragas, Andrea V.UTNFRDnanomechanicsultrafast opticsnanoantennaspolymersplasmonicsNanotechnology and the consequent emergence of miniaturized devices are driving the need to improve our understanding of the mechanical properties of a myriad of materials. Here we focus on amorphous polymeric materials and introduce a new way to determine the nanoscale mechanical response of polymeric thin films in the GHz range, using ultrafast optical means. Coupling of the films to plasmonic nanoantennas excited at their vibrational eigenfrequencies allows the extraction of the values of the mechanical moduli as well as the estimation of the glass transition temperature via time-domain measurements, here demonstrated for PMMA films. This nanoscale method can be extended to the determination of mechanical and elastic properties of a wide range of spatially strongly confined materials.Fil: Scarpettini, Alberto F. Universidad Tecnológica Nacional. Facultad Regional Delta. Grupo Nanofotonica; Argentina.Peer Reviewed2020-09-18T18:27:36Z2020-09-18T18:27:36Z2020-06-02info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfDetermination of Nanoscale Mechanical Properties of Polymers via Plasmonic Nanoantennas Hilario D. Boggiano, Rodrigo Berté, Alberto F. Scarpettini, Emiliano Cortés, Stefan A. Maier, and Andrea V. Bragas ACS Photonics 2020 7 (6), 1403-1409 DOI: 10.1021/acsphotonics.0c00631http://hdl.handle.net/20.500.12272/455110.1021/acsphotonics.0c00631enghttps://pubs.acs.org/doi/abs/10.1021/acsphotonics.0c00631info:eu-repo/semantics/openAccess2020-09-18T18:27:36Zhttp://creativecommons.org/licenses/by-nc-sa/4.0/Atribución-NoComercial-CompartirIgual 4.0 InternacionalScarpettini, AlbertoAtribución – No Comercial – Compartir Igual (by-nc-sa)reponame:Repositorio Institucional Abierto (UTN)instname:Universidad Tecnológica Nacional2026-09-24T12:48:44Zoai:ria.utn.edu.ar:20.500.12272/4551instacron:UTNInstitucionalhttp://ria.utn.edu.ar/Universidad públicaNo correspondehttp://ria.utn.edu.ar/oaigestionria@rec.utn.edu.ar; fsuarez@rec.utn.edu.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:a2026-09-24 12:48:45.449Repositorio Institucional Abierto (UTN) - Universidad Tecnológica Nacionalfalse
dc.title.none.fl_str_mv Determination of Nanoscale Mechanical Properties of Polymers via Plasmonic Nanoantennas
title Determination of Nanoscale Mechanical Properties of Polymers via Plasmonic Nanoantennas
spellingShingle Determination of Nanoscale Mechanical Properties of Polymers via Plasmonic Nanoantennas
Boggiano, Hilario D
UTN
FRD
nanomechanics
ultrafast optics
nanoantennas
polymers
plasmonics
title_short Determination of Nanoscale Mechanical Properties of Polymers via Plasmonic Nanoantennas
title_full Determination of Nanoscale Mechanical Properties of Polymers via Plasmonic Nanoantennas
title_fullStr Determination of Nanoscale Mechanical Properties of Polymers via Plasmonic Nanoantennas
title_full_unstemmed Determination of Nanoscale Mechanical Properties of Polymers via Plasmonic Nanoantennas
title_sort Determination of Nanoscale Mechanical Properties of Polymers via Plasmonic Nanoantennas
dc.creator.none.fl_str_mv Boggiano, Hilario D
Berté, Rodrigo
Scarpettini, Alberto F
Cortés, Emiliano
Maier, Stefan A.
Bragas, Andrea V.
author Boggiano, Hilario D
author_facet Boggiano, Hilario D
Berté, Rodrigo
Scarpettini, Alberto F
Cortés, Emiliano
Maier, Stefan A.
Bragas, Andrea V.
author_role author
author2 Berté, Rodrigo
Scarpettini, Alberto F
Cortés, Emiliano
Maier, Stefan A.
Bragas, Andrea V.
author2_role author
author
author
author
author
dc.subject.none.fl_str_mv UTN
FRD
nanomechanics
ultrafast optics
nanoantennas
polymers
plasmonics
topic UTN
FRD
nanomechanics
ultrafast optics
nanoantennas
polymers
plasmonics
dc.description.none.fl_txt_mv Nanotechnology and the consequent emergence of miniaturized devices are driving the need to improve our understanding of the mechanical properties of a myriad of materials. Here we focus on amorphous polymeric materials and introduce a new way to determine the nanoscale mechanical response of polymeric thin films in the GHz range, using ultrafast optical means. Coupling of the films to plasmonic nanoantennas excited at their vibrational eigenfrequencies allows the extraction of the values of the mechanical moduli as well as the estimation of the glass transition temperature via time-domain measurements, here demonstrated for PMMA films. This nanoscale method can be extended to the determination of mechanical and elastic properties of a wide range of spatially strongly confined materials.
Fil: Scarpettini, Alberto F. Universidad Tecnológica Nacional. Facultad Regional Delta. Grupo Nanofotonica; Argentina.
Peer Reviewed
description Nanotechnology and the consequent emergence of miniaturized devices are driving the need to improve our understanding of the mechanical properties of a myriad of materials. Here we focus on amorphous polymeric materials and introduce a new way to determine the nanoscale mechanical response of polymeric thin films in the GHz range, using ultrafast optical means. Coupling of the films to plasmonic nanoantennas excited at their vibrational eigenfrequencies allows the extraction of the values of the mechanical moduli as well as the estimation of the glass transition temperature via time-domain measurements, here demonstrated for PMMA films. This nanoscale method can be extended to the determination of mechanical and elastic properties of a wide range of spatially strongly confined materials.
publishDate 2020
dc.date.none.fl_str_mv 2020-09-18T18:27:36Z
2020-09-18T18:27:36Z
2020-06-02
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv Determination of Nanoscale Mechanical Properties of Polymers via Plasmonic Nanoantennas Hilario D. Boggiano, Rodrigo Berté, Alberto F. Scarpettini, Emiliano Cortés, Stefan A. Maier, and Andrea V. Bragas ACS Photonics 2020 7 (6), 1403-1409 DOI: 10.1021/acsphotonics.0c00631
http://hdl.handle.net/20.500.12272/4551
10.1021/acsphotonics.0c00631
identifier_str_mv Determination of Nanoscale Mechanical Properties of Polymers via Plasmonic Nanoantennas Hilario D. Boggiano, Rodrigo Berté, Alberto F. Scarpettini, Emiliano Cortés, Stefan A. Maier, and Andrea V. Bragas ACS Photonics 2020 7 (6), 1403-1409 DOI: 10.1021/acsphotonics.0c00631
10.1021/acsphotonics.0c00631
url http://hdl.handle.net/20.500.12272/4551
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv https://pubs.acs.org/doi/abs/10.1021/acsphotonics.0c00631
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
2020-09-18T18:27:36Z
http://creativecommons.org/licenses/by-nc-sa/4.0/
Atribución-NoComercial-CompartirIgual 4.0 Internacional
Scarpettini, Alberto
Atribución – No Comercial – Compartir Igual (by-nc-sa)
eu_rights_str_mv openAccess
rights_invalid_str_mv 2020-09-18T18:27:36Z
http://creativecommons.org/licenses/by-nc-sa/4.0/
Atribución-NoComercial-CompartirIgual 4.0 Internacional
Scarpettini, Alberto
Atribución – No Comercial – Compartir Igual (by-nc-sa)
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.source.none.fl_str_mv reponame:Repositorio Institucional Abierto (UTN)
instname:Universidad Tecnológica Nacional
reponame_str Repositorio Institucional Abierto (UTN)
collection Repositorio Institucional Abierto (UTN)
instname_str Universidad Tecnológica Nacional
repository.name.fl_str_mv Repositorio Institucional Abierto (UTN) - Universidad Tecnológica Nacional
repository.mail.fl_str_mv gestionria@rec.utn.edu.ar; fsuarez@rec.utn.edu.ar
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score 13.24418